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Great question—certainly if you rapidly cool an aerogel the thermally-induced stresses throughout the material could exacerbate fracture.

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Some aerogels, made the right way, are certainly sustainable! To develop a true estimate of the volume of return flow, an estimate of the evaporative effect must be included. It would appear Prof James Hardy of the Doqnload of Akron has discontinued his two semester online chemistry tutorials!

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